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Nanophotonics and Nanoelectronics
Jerry Simmons, SNL
Victor Klimov, LANL

Description: The Nanophotonics and Nanoelectronics theme will be built upon capabilities needed to control electronic and photonic properties of nanostructured materials. The capabilities will be targeted at the overall scientific challenge of understanding and controlling fundamental electronic and photonic interactions in nanostructured materials, which will require achieving control of material properties at the level of electron and photon wavefunctions. The thrust area will support user programs, both in nanophotonics and nanoelectronics and in areas that require the integration of capabilities from this thrust with other CINT thrusts. The scientific challenges to be addressed will include developing nanostructures significantly more complex than existing materials, incorporating multiple constituents, finer length scales, and new 3D architectures. These complex nanostructures will exhibit unique electronic and optical properties that will enable a new generation of miniature, multifunctional, high performance devices. The research will be strongly supported by an effort in instrument development with an emphasis on ultra-pure semiconductor growth with atomic precision, and on new characterization tools that will allow monitoring of electronic phenomena with atomic-scale spatial resolution.

The research topics that will be addressed include:
1) control and manipulation of charge, spin, and wave functions in individual nanostructures and assemblies of únanoblocksî of various complexities,
2) single-electron quantum transport including electron spin and its implications for quantum computing,
3) single-electron memory arrays,
4) functional circuits comprising arrays of molecular transistors,
5) photon harvesting nanostructures for energy conversion and catalysis,
6) úactiveî photonic nanostructures for optical amplification, ultrafast optical switching and chem/bio sensing, and 7) photonic lattices for high bandwidth optical communications and computing.

Key equipment and facilities at full operation:
  • Multi-use clean room for processing of a wide variety of materials. It will include photolithography, metal deposition, etching tools and characterization equipment.
  • Electron beam lithography capabilities for top-down patterning of nanostructures and integration with larger structures.
  • Molecular beam epitaxy for growth of ultra-high purity compound semiconductor heterostructures enabling well defined single electron energy levels
  • General use transport labs for both dc and high frequency electrical measurements at low (milliKelvin) temperature and high magnetic fields.
  • Wet-chemistry laboratory for fabrication (synthesis and assembly) of organic and inorganic nanostructured materials including colloidal quantum dots, synthetic opal structures, organic/inorganic multilayers, light-harvesting nanoassemblies, etc.
  • Facilities for high-spatial resolution imaging and spectroscopy using úregularî and úadvancedî scanning probes; úadvancedî probes include an ultrafast scanning tunneling microscope (STM), a transient absorption, near-field scanning optical microscope/spectrometer (NSOM), and a magnetic resonance-force microscope.
  • Facilities for state-of-the-art single molecule/nanostructure and ultrafast optical and THz spectroscopies.

    Equipment and facilities at startup:
  • Facility for semiconductor growth and electron beam lithography.
  • Cryogenic facilities for low-temperature and high-magnetic-field electrical and optical measurements.
  • Energetic neutral atom beam epitaxy for high-spatial resolution etching and thin film growth.
  • Wet-chemistry laboratory for colloidal synthesis.
  • Optical spectroscopy and microscopy instrumentation including capabilities for time-resolved measurements.
  • Facilities and capabilities for scanning tunneling, atomic-force and near-field microscopies.

    Programs and personnel at startup: A number of existing programs will be used to support the capabilities of the thrust during the CINT startup phase. Within these programs, specific scientific areas that are being explored include:
    1) Active assembly of photonic nanostructures,
    2) Self-assembly of nanostructures,
    3) Coulomb interactions and quantum (phase) interference of electrons in coupled lower dimensional semiconductor structures,
    4) Superparamagnetic transition in shape controlled magnetic nanoparticles,
    5) Development of ultrafast STM and NSOM, and
    6) Energy transfer through assemblies of nanostructured components.

    Key personnel who will contribute to the thrust area include the thrust leaders and the PIs of leveraged programs (V. I. Klimov, J. Simmons, A. Taylor, M. Lilly, S. Lin, M. Sinclair, J. Reno, D. Smith, M. Hoffbauer, J. Wendt, and S. Trugman).

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    January 29, 2003